Neisseria gonorrhoeae causes the sexually transmitted disease gonorrhea, which has a global incidence of 106 million cases per year. No vaccine is available to prevent the disease, and the emergence of multidrug resistant (MDR) strains makes N. gonorrhoeae an immediate public health threat. Here, we show that the chemical synergy between an ionophore, PBT2 and zinc can reverse the intrinsic resistance of N. gonorrhoeae to cationic antibiotic peptides polymyxin B or colistin. PBT/zinc can also increase the susceptibility of N. gonorrhoeae to two cationic antimicrobial peptides, LL-37 and PG-1, which are naturally present in mammals. The emergence of bacterial strains that are resistant to available antimicrobials is a current health emergency. Treatment with PBT2/zinc to sensitize the bacterium to antimicrobial peptides may represent a new strategy to treat MDR N. gonorrhoeae infections and reinvigorate the use of currently available antibiotics.